APPROCHES SYNTHETIQUES ALTERNATIVES ET COMPLEMENTAIRES VERS LES ARISTOLACTAMES

  • RYBALKO-ROSEN HÉLÉNE
    UNIVERSITÏ¿½ DES SCIENCES ET TECHNOLOGIES DE LILLE 1, F-59655 VILLENEUVE D`ASCQ CÏ¿½DEX, FRANCE
  • COUTURE AXEL
    UNIVERSITÏ¿½ DES SCIENCES ET TECHNOLOGIES DE LILLE 1, F-59655 VILLENEUVE D`ASCQ CÏ¿½DEX, FRANCE
  • GRANDCLAUDON PIERRE
    UNIVERSITÏ¿½ DES SCIENCES ET TECHNOLOGIES DE LILLE 1, F-59655 VILLENEUVE D`ASCQ CÏ¿½DEX, FRANCE

Abstract

Two conceptually new synthetic approaches to alkaloids aristolactam has been developed. They differ from the synthetic tactics employed for the construction of common precursors i.e. haloarylmethylene isoindolinones. These highly conjugated systems have been obtained by Horner reaction or E1cb elimination involving phosphorylated or dephosphorylated isoindolinones respectively. Free radical cyclization completes the synthesis of the target fused aristolactams.

Cuvinte cheie

alkaloids aristolactams radical cyclization Horner reaction aryne enamides