REACTIVTE DES PYRANES - SYNTHESE DE NOUVEAUX HETEROCYCLES POLYNUCLEAIRES CONDENSES: PYRIDINOPYRANES FONCTIONNALISES ET PYRIMIDINOPYRIDINOPYRANES

  • HAFIDH AFIFA
    LABORATOIRE DE CHIMIE DE LA MATIÈRE CONDENSÉE, INSTITUT PRÉPARATOIRE AUX ETUDES D’INGÉNIEURS DE TUNIS
    AFIFA.HAFIDH@IPEIT.RNU.TN
  • GHARBI NEJI
    LABORATOIRE DE CHIMIE DE LA MATIÈRE CONDENSÉE, INSTITUT PRÉPARATOIRE AUX ETUDES D’INGÉNIEURS DE TUNIS

Abstract

Aminocyanopyranes 1 react respectively with diethylmalonate, acetylacetone and ethylacetoacetate to give the corresponding functional pyranopyridines 2, 3 and 4. The reaction of the compounds 2, 3 and 4 with orthoesters then with primary amines affords respectively the pyranopyridinopyrimidines 5, 7 and 8. Refluxing of the functional pyranopyridines 2 with hydrazine in ethanol leads to the pyrimidinohydrazinopyridinopyranes 6. The structures of all prepared products were determined on the basis of their IR, 1H and 13C NMR spectra.

Cuvinte cheie

pyrane pyranopyridine pyrimidine pyridinopyrimidine pyranopyridinopyrimidine aminopyridopyrane